arXiv Daily: nickelate superconductors 2026-02-05
Daily Overview: Today’s highlight focuses on advancing the understanding of the electronic structure of hybrid Ruddlesden-Popper nickelates. Using Raman scattering spectroscopy, the research team comprehensively characterized the electronic, magnetic, and lattice excitations of the bilayer nickelate La₃Ni₂O₇ under ambient pressure. For the first time, they simultaneously observed two types of in-plane spin exchange interactions along the Ni-O bond direction and the diagonal direction in the spin-density-wave state, revealing the bond-diagonal antiferromagnetic competition mediated by the nickel d_{x²-y²} orbitals. Moreover, the discovery of low-energy two-magnon excitations provides direct spectroscopic evidence for spin disproportionation, while anomalous phonon softening hints at an incipient lattice instability. These results collectively establish the correlation among competitive spin interactions, spin disproportionation, and lattice response in this system, providing key experimental foundations for understanding the microscopic mechanism of nickelate superconductivity. arXiv submission processing window: 2026-02-05 06:39 to 2026-02-05 06:39 UTC. ...