arXiv Daily: nickelate superconductors 2026-02-24
Daily Overview: The highlight of today’s work focuses on an in-depth understanding of the electronic structure of mixed Ruddlesden-Popper nickelates. In [1], DFT and RPA calculations revealed an s±-wave pairing mechanism in the bilayer subsystem of high-pressure La₅Ni₃O₁₁, where the monolayer subsystem is coupled to the bilayer via weak interlayer Josephson coupling, naturally explaining the dome-shaped Tc-pressure relationship and highlighting the distinct pressure response of mixed-phase compared to pure-phase nickelates. [2] proposes that applying a perpendicular electric field in La₃Ni₂O₇ single-double layer thin films can drive charge transfer, increasing the filling rate and thereby enhancing intralayer d-wave pairing, with theoretical predictions that Tc could exceed the liquid nitrogen temperature (~77 K), providing a new pathway for achieving high-temperature superconductivity at ambient pressure. [3] systematically constructs the superconducting phase diagram of multilayer square-planar nickelates Nd_{n+1}Ni_nO_{2n+2} (n = 4–8), achieving a maximum onset Tc of 12.9 K (n = 6), with magnetic fluctuations persisting in the superconducting region and the superconducting regime overlapping with that of infinite-layer nickelates, offering a template for atomic-precision layered design. [4] points out that in pressurized Ruddlesden-Popper nickelates, the incorrect formula used has systematically overestimated the superconducting volume fraction by approximately a factor of two (actual value only 51–59%), calling for recalculation using the correct equation, thus providing an important correction to the reliability of related experimental data. arXiv submission processing window: 2026-02-24 00:00 to 2026-02-24 00:00 UTC. ...