Daily Overview: Today’s highlighted work focuses on a deeper understanding of the electronic structure of mixed-type Ruddlesden-Popper nickelates. On the theoretical side, [1] combines variational Monte Carlo calculations within an effective five-layer Hubbard model and finds that the spin-singlet d_{x^2-y^2}-wave state of La6Ni5O12 is energetically favored while extended s-wave pairing is strongly suppressed; based on the optimized superconducting state, [1] predicts signatures of a clean nodal superconductor, including a V-shaped tunneling density of states, linear depletion of the low-temperature superfluid density, a decrease in the Knight shift below Tc, and 1/(T1T)∝T^2. Within the same framework, LaNiO2 shows a robust d-wave tendency, and La4Ni3O8 lies close to the boundary between d-wave superconducting and non-superconducting states; on this basis, [1] proposes that a common d_{x^2-y^2}-wave pairing tendency may exist in the reduced RP nickelate family but emphasizes that this remains a theoretical prediction rather than an experimental establishment. On the experimental side, [2] uses 139La NQR spectra of La3Ni2O7.0 at ambient pressure combined with DFT+U calculations, observes two La(2)a/La(2)b sites with near-1:1 occupancy, points out that the two intrinsic inequivalent La(2) sites and two inequivalent Ni sites in the low-symmetry Am2m (No.38) structure naturally explain this phenomenon, and rules out defect models attributing the signal to stacking faults, impurity phases, or oxygen vacancies; based on the Am2m framework, [2] identifies the commensurate SDW state as “large-small spin stripe” order, in which different internal fields are associated with the small magnetic moment at Nia and the larger magnetic moment at Nib, respectively, and the small-spin Ni site has higher electron occupancy but a smaller magnetic moment, inconsistent with the local-moment picture, indicating that the ambient-pressure SDW order is driven by Fermi-surface nesting and is itinerant in nature. On the model side, [3] performs finite-temperature determinant quantum Monte Carlo simulations of a single-orbital bilayer Hubbard model under conditions of strong interlayer coupling and comparable intralayer and interlayer antiferromagnetic correlation strengths, showing that spin stripes form spontaneously with increasing hole doping and that the dominant pairing symmetry crosses from d-wave to s±-wave; this crossover tracks changes in the relative strengths of the two types of spin correlations, and the odd-channel dynamic spin structure factor further exhibits momentum-dependent reorganization of magnetic excitations. On this basis, [3] considers the spin-fluctuation structure to be a key link connecting spin stripes and pairing competition, providing a minimal-model perspective for understanding La3Ni2O7, although this result is a model-calculation prediction rather than an established experimental mechanism. arXiv submission processing window: 2026-11-05 00:00 to 2026-11-05 00:00 UTC.
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