arXiv Daily: Nickelate superconductors 2026-05-05
Daily Overview: Here is the English translation of the provided Chinese daily paper overview: > — > Today’s Research Overview in the Nickelate Superconductor Field > Two research works today deepen our understanding of the superconducting mechanism in layered nickel oxides from the perspectives of structural and electronic phase transitions, as well as the relationship between electronic ordered phases and superconductivity. > First, a team from Université Paris-Saclay and other institutions systematically mapped the temperature-pressure phase diagram of the bilayer nickelate La₃Ni₂O₇ using high-pressure high-temperature Raman and infrared spectroscopy. They discovered that a pressure-induced lattice tilt-to-untilt structural phase transition is accompanied by a nearly two-order-of-magnitude increase in carrier concentration, and superconductivity is observed near the phase boundary. This work establishes a direct link between structural and electronic property changes, providing a key experimental foundation for understanding its high-pressure superconducting mechanism. > Meanwhile, another study led by Brookhaven National Laboratory and other institutions focuses on bilayer nickelate La₂PrNi₂O₇ thin films. Using resonant X-ray scattering and spectroscopy, they provide strong evidence that the spin density wave (SDW) is not a precursor state of superconductivity but rather a competing phase associated with oxygen vacancies. The work further proposes that in the superconducting phase, regions with intact oxygen stoichiometry have a ground state characterized by robust interlayer five-spin polaron states, which lock out-of-plane orbitals and render the in-plane orbital behavior close to the classical electronic configuration of cuprates and infinite-layer nickelates. > In summary, these studies not only elucidate the structural origin of pressure-driven superconductivity but also reveal the key regulatory role of oxygen stoichiometry in electronic states and the superconducting/competing phase balance, offering new perspectives for exploring the microscopic mechanism of nickelate superconductivity. ...