Daily Overview: This post sorts papers by relevance to nickelate superconductors. Summaries are AI-generated and may contain errors. arXiv submission processing window: times are unavailable (UTC).
1. Decoding Superconductivity in La$_3$Ni$_2$O$_{7-δ}$ Thin Films via Ozone-Driven Structure and Oxidation Tuning
- Relevance Score:
5.8745 - Authors: Mathieu Flavenot, Hoshang Sahib, Jérôme Robert, Marc Lenertz, Gilles Versini, Laurent Schlur, Alexandre Gloter, Nathalie Viart, Daniele Preziosi
- Affiliations: Université de Strasbourg, Université Paris-Saclay
- Link: http://arxiv.org/abs/2604.09807v1
- Paper page: Decoding Superconductivity in La₃Ni₂O₇-δ Thin Films via Ozone-Driven Structure and Oxidation Tuning
Summary: This study presents a detailed structural analysis of epitaxial La₃Ni₂O₇₋δ thin films using scanning transmission electron microscopy combined with electron energy loss spectroscopy. The films were prepared on SrLaAlO₄ substrates via pulsed laser deposition and exhibited significantly distinct superconducting properties after different ozone annealing treatments. It was found that the stabilization of the superconducting phase is closely related to oxygen stoichiometry uniformity, epitaxial strain, and specific stacking structural motifs such as bilayers and polytypes. By correlating the rich morphology of stacking polytypes with transport behavior, a theoretical framework for understanding metastable superconducting phases in bilayer nickelate thin films was established. The results reveal the critical roles of oxygen content, lattice strain, and structural ordering in achieving ambient-pressure superconductivity, providing a clear pathway for designing new nickel-based superconducting materials.
2. High-temperature superconductivity in Nd$_{0.85}$Sr$_{0.15}$NiO$_2$ membranes under pressure
- Relevance Score:
5.1582 - Authors: Yonghun Lee, Mengnan Wang, Xin Wei, Yijun Yu, Wendy L. Mao, Yu Lin, Harold Y. Hwang
- Affiliations: SLAC National Accelerator Laboratory, Stanford University, Fudan University
- Link: http://arxiv.org/abs/2604.09525v1
- Paper page: High-temperature superconductivity in Nd₀.85Sr₀.15NiO₂ membranes under pressure
Summary: Researchers have developed a technique to integrate free-standing infinite-layer Nd₀.₈₅Sr₀.₁₅NiO₂ thin films into diamond anvil cells, thereby overcoming the difficulties of measuring such films under high-pressure conditions. By applying pressures up to approximately 90 GPa to the films, they observed that the superconducting transition temperature (T_c) increased monotonically and linearly from about 17 K at ambient pressure to roughly 74.2 K, with an enhancement rate of approximately 0.65 K/GPa and no signs of saturation. This linear, non-saturating pressure dependence of T_c markedly differs from the pressure-induced overdoping that leads to T_c suppression in most copper oxide superconductors and bilayer nickelates, suggesting that the pairing strength in infinite-layer nickelates can be elevated to unexpectedly high levels. Furthermore, measurements of the upper critical field and coherence length confirm the pressure-induced enhancement of the superconducting state. This study provides a new pathway for continuously enhancing superconductivity through lattice compression, and the developed free-film high-pressure technique holds promise for broad application to other two-dimensional materials.