Daily Overview: This post sorts papers by relevance to nickelate superconductors. Summaries are AI-generated and may contain errors. arXiv submission processing window: times are unavailable (UTC).
1. Dissecting superconductivity in the Ruddlesden-Popper nickelates: The role of electron correlation and interlayer magnetic exchange
- Relevance Score:
5.7332 - Authors: Xiaoyang Chen, Zezhong Li, Mei Xie, Deyuan Hu, Yiu-Fung Chiu, Stefano Agrestini, Wenliang Zhang, Yi Lu, Meng Wang, Mirian Garcia-Fernandez, Donglai Feng, Ke-Jin Zhou
- Link: http://arxiv.org/abs/2604.01902v1
- Paper page: Dissecting superconductivity in the Ruddlesden-Popper nickelates: The role of electron correlation and interlayer magnetic exchange
Summary: This study employs resonant inelastic X-ray scattering (RIXS) to directly compare the electronic and magnetic excitation properties of trilayer nickelate La₄Ni₃O₁₀ and bilayer La₃Ni₂O₇. The results show that La₄Ni₃O₁₀ exhibits more itinerant behavior, evidenced by broader Ni d-d orbital excitations and a stronger fluorescence background, indicating weaker electronic correlations than in the bilayer system. Despite the weaker correlations, clear collective spin excitations are observed, including dispersive acoustic and optical magnon branches as well as incommensurate spin density waves (SDW). Using linear spin-wave theory analysis, the interlayer superexchange interaction Jz is extracted to be approximately 22 meV, significantly smaller than that in La₃Ni₂O₇. The weaker electron correlations and reduced interlayer magnetic exchange together account for the substantially lower superconducting transition temperature of the trilayer compound (about 30 K) compared to the bilayer (about 80 K). This study establishes interlayer magnetic coupling and electronic correlations as key parameters for superconductivity in layered nickelates, providing important constraints for understanding the superconducting pairing mechanism in this emerging family.
2. Jahn-Teller distortion on strained La$_3$Ni$_2$O$_7$ thin films
- Relevance Score:
5.4859 - Authors: Yuxin Wang, Zhan Wang, Fu-Chun Zhang, Kun Jiang
- Link: http://arxiv.org/abs/2604.02191v2
- Paper page: Jahn-Teller distortion on strained La₃Ni₂O₇ thin films
Summary: This study systematically analyzed the electronic structure of strained La₃Ni₂O₇ thin films using density functional theory calculations, revealing that biaxial compressive strain primarily elongates the outer apical Ni–O bonds while leaving the inner apical Ni–O bonds nearly unchanged, thereby significantly enhancing the Jahn–Teller splitting energy Δ_JT, yet the interlayer d_z² orbital hopping parameter t_⊥^z exhibits only a weak variation. Given that superconductivity emerges only when the in-plane lattice constant falls below a critical value, these results identify strain-enhanced Δ_JT as a key microscopic tuning parameter. The calculated Fermi surface topology and Hall response agree well with angle-resolved photoemission spectroscopy (ARPES) and Hall measurements on LaAlO₃ and SrLaAlO₄ substrates, confirming that Jahn–Teller distortion plays a central role in optimizing superconductivity in bilayer nickelates.